Proton Guns Set Their Sights on Taming Radioactive WastesDennis Normile
Once mooted as energy sources, nuclear reactors that substitute particle accelerators for chain reactions are taking long-range aim at a new mission
KUMATORI, JAPAN--On the grounds of Kyoto University's Research Reactor Institute, workers have dug into a hillside to give a 30-year-old experimental nuclear reactor an unusual companion: a proton synchrotron. When it starts up in fall 2005, the synchrotron will fire protons into the heart of the reactor, straight down the axis of a cylinder of heavy metal wrapped in a core of nuclear fuel. Neutrons dislodged from the target will hurtle into the fuel, shattering atoms as they go.
It may seem a roundabout way to generate a nuclear reaction, and it is. But this type of accelerator-driven system (ADS), as it's called, isn't primarily designed to generate power. Instead, its aim is to transform some of the nastier ingredients of spent reactor fuel into less troublesome elements. The technology "has a unique role to play in treating nuclear wastes," says Stefano Monti, a nuclear physicist at the Italian National Agency for New Technologies, Energy, and the Environment (ENEA) in Rome.
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The basic processes at work in an ADS--splitting atoms to change one element into another--have been understood for almost a century. Similar schemes were briefly studied in the 1950s to turn thorium into uranium-235 to fuel nuclear reactors. The idea was revived in the 1980s when scientists started wrestling with the problem of waste from nuclear power plants. The most troublesome components of nuclear waste are long-lived fission products and actinides --elements such as americium and curium --which have half-lives of thousands of years. Researchers working separately at Brookhaven National Laboratory in Upton, New York, and at Los Alamos started looking at using subcritical, or non-self-sustaining, nuclear reactions to burn up these wastes. They envisioned using an accelerator to fire a beam of protons at a target surrounded by spent nuclear fuel. In what is called a spallation reaction, the protons break target nuclei, producing neutrons that trigger reactions in the surrounding material (see figure). Some radioactive elements are rendered nonradioactive. Others absorb a neutron, become unstable, and then either fission or decay. Actinides, for example, are transmuted into uranium, which decays into shorter-lived radionuclides that can be disposed of as low-level nuclear waste. Because the reaction is subcritical, if the stream of protons is shut off, the reaction stops.
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http://www.sciencemag.org/cgi/content/full/302/5644/379